If there is a radio spectrum issue or a deeper down networking issue, replacing the gear may not solve the problem. So I’d try to isolate the current setup’s issue before blindly replacing it.
A wired backhaul is always going to provide better performance, reliability, and consistency… as well as the lowest latency. Wireless backhaul is going to be more problematic in a radio-heavy area, or if your building has a lot of dense materials. But otherwise a wireless backhaul may be perfectly suitable for your needs.
Four nodes can be a lot. The most nodes I have installed is three, in homes that are about 4500 sq ft. These are in modern North American “wood & drywall” homes, and I was able to position the nodes well, so your situation may demand something else. Generally I want to use as few nodes as I can, because there is a system performance overhead for each node.
6 GHz is great if you have a lot of 6E gear, but it is worse than 5 GHz in terms of traversing walls and materials. So if you have an open floorplan it’s a good option, but otherwise I’d save my money. I only have one 6e kit installed in a home, and there has been at most one client I’ve seen connected to 6 GHz. The backhaul prefers 5 GHz.
Yes. Maybe turn off/disable the WiFi radio on your older modem so that the new router isn’t impacted by the radio noise from the old modem.